Im a self made learner from repairing my 71 Cuda grille. You are correct: That plastic is as brittle as it comes.
I learned from repairing all sorts of composite grilles. And the absolute best thing I have EVER used to repair, to inlude my 71 grill, was plain fiberglass repair resin, WITHOUT the matting
To do this right, you need to remove the grill:
-Remove front valance, remove front bumper. Then loosen the center front bumper mounts that attach to the frame (You will need to for the extra inch or so clearanace to remove /reinstall the front grill)
You DONT have to remove the headlight bezels. Reomve all bolts holding the grill on. Dont forget the one on each side, bottom corners of the grill
Remove grille carefully
On all my cracks, where the crack stopped, I did drill a hole, very very small so the crack would not extend any further. Repairing one crack at a time is the key= taking your time
I did my repairs on the blind side, not visible from the outside world
After drilling the small hole, I took 600 grit and lightly sanded on the crack and about a half inch out on the surface that I would repair. Apply a piece of tape on the other side of the crack: Mix the resin, and apply to the crack: Use gravity to help you as you apply this stuff: It will run if you dont, (Thats why you have the peice of tape on the down side): Position the grill so that you leave a "pool" of resin over the crack: Let it cure about an hour I didnt even sand the resin when cured
But on the side that you can see when the grill is mounted, youll need to use some glazing compound to fill the crack for cosmetic reasons, then paint over the repair
I then painted my grill with the closet match that I could to the original "silver"
When you have the grill off, look VERY carefully for other cracks. I gaurenntee you have more than one crack present